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High refractive index dielectrics enable nanoscale integration of optical components with practically no absorption loss. Hence, high index dielectrics are promising for many emerging applications in nanophotonics. However, the lack of a complete library of high index dielectric materials poses a significant challenge to understanding the full potential for dielectric nanophotonics. Currently, it is assumed that the absorption edge and the sub‐bandgap refractive index of a semiconductor exhibit a rigid trade‐off, popularly known as the Moss rule. Thus, the Moss rule appears to set an upper limit on the refractive index of a dielectric for a given operating wavelength. However, there are many dielectric materials that surpass the Moss rule, referred to here as super‐Mossian dielectrics. Here, the general features of super‐Mossian dielectrics and their physical origin are discussed to facilitate the search for high index dielectrics. As an example, iron pyrite, an outstanding super‐Mossian material with index nearly 40% higher than the Moss rule prediction, is developed. The local dielectric resonances in iron pyrite nanoresonators are experimentally observed, and the impact of super‐Mossian materials on nanophotonics is demonstrated.

All open systems that exchange energy with their environment are non‐Hermitian. Thermal emitters are open systems that can benefit from the rich set of physical phenomena enabled by their non‐Hermitian description. Using phase, symmetry, chirality, and topology, thermal radiation from hot surfaces can be unconventionally engineered to generate light with new states. Such thermal emitters are necessary for a wide variety of applications in sensing and energy conversion. Here, a non‐Hermitian selective thermal emitter is experimentally demonstrated, which exhibits passivePT‐symmetry in thermal emission at 700 °C. Furthermore, the effect of internal phase of the oscillator system on far‐field thermal radiation is experimentally demonstrated. The ability to tune the oscillator phase provides new pathways for both engineering and controlling selective thermal emitters for applications in sensing and energy conversion.